Electrochemical Behavior, Structure, and Morphology of Electrodeposited Nickel on Copper Alloy Prepared from Sulfate Bath without Additive Addition

Bambang Soegijono, Ferry Budhi Susetyo, Hamdan Akbar Notonegoro, Musfirah Cahaya Fajrah

Abstract


Nickel and nickel alloy has good chemical and physical properties to enhance corrosion resistance. Electrodeposited nickel layer are expected to enhance corrosion resistance of copper as substrates. The difference distance crystal plane of Nickel and Copper is about 0.02 – 0.03 Angstrom. The electrochemical behavior, structure and morphology of electrodeposited nickel on copper substrate in sulfate solution were investigated. Electrodepositions of nickel layer were conducted at room temperature with various current densities (10 mA/cm², 20 mA/cm², and 30 mA/cm²). Electrochemical behavior, structure, and morphology of the samples were analyzed by using potensiostat, x-ray diffraction (XRD), and Scanning electron microscope (SEM). The x-ray diffraction patterns show that the nickel has cubic FCC crystal system and space group Fm-3m.  The current density during electrodeposition influence crystal parameter, crystallite size and micro strain of nickel film deposited. Electrodeposited nickel with current density 30 m A/cm² shows the best corrosion resistance.

Keywords


Nickel, Copper alloy, Electro-deposition, Sulfate solution

Full Text:

PDF

References


Ming Z, Chunkai L, Gang Z, Yu S, Ding F, Jiankang H. Modeling and control of consumable DE-GMAW process. J Manuf Process. 2016;24:293–7.

Chai Z, Jiang C, Zhao Y, Wang C, Zhu K, Cai F. Microstructural characterization and corrosion behaviors of Ni-Cu-Co coatings electrodeposited in sulphate-citrate bath with additives. Surf Coatings Technol. 2016;307:817–24.

Thurber CR, Ahmad YH, Sanders SF, Al-Shenawa A, D’Souza N, Mohamed AMA, et al. Electrodeposition of 70-30 Cu-Ni nanocomposite coatings for enhanced mechanical and corrosion properties. Curr Appl Phys. 2016;16(3):387–96.

Abdulwahab M, Fayomi OSI, Popoola API. Structural evolution, thermomechanical recrystallization and electrochemical corrosion properties of Ni-Cu-Mg amorphous coating on mild steel fabricated by dual-anode electrolytic processing. Appl Surf Sci. 2016;375:162–8.

Wang J, Xu J, Zhang X, Ren X, Song X, Chen X. An investigation of surface corrosion behavior of Inconel 718 after robotic belt grinding. Materials (Basel). 2018;11(12):1–14.

Genna S, Trovalusci F, Ucciardello N, Tagliaferri V. Improving performance of an open cell aluminium foam through electro-deposition of nickel. Materials (Basel). 2019;12(1).

Riyanto, Rofida I. Preparation and application of nickel plating on copper electrode (NPCE) for uric acid analysis in human urine using cyclic voltammetry. Int J Electrochem Sci. 2019;14(3):2290–304.

Zhao H, Liu L, Zhu J, Tang Y, Hu W. Microstructure and corrosion behavior of electrodeposited nickel prepared from a sulphamate bath. Mater Lett. 2007;61(7):1605–8.

Jinlong L, Yang M, Suzuki K, Miura H, Zhang Y. Comparison of corrosion resistance of electrodeposited pure Ni and nanocrystalline Ni–Fe alloy in borate buffer solution. Mater Chem Phys. 2017;202:15–21.

Zhu Z, Zhu D, Qu N. Effects of simultaneous polishing on electrodeposited nanocrystalline nickel. Mater Sci Eng A. 2011;528(24):7461–4.

Cheng W, Ge W, Yang Q, Qu X. Study on the corrosion properties of nanocrystalline nickel electrodepositied by reverse pulse current. Appl Surf Sci. 2013;276:604–8.

López JR, Stremsdoerfer G, Trejo G, Ortega R, Pérez JJ, Meas Y. Corrosion Resistance of Nickel Coatings Obtained by Electrodeposition in a Sulfamate Bath in the Presence of Samarium ( III ). Int J Electrochem Sci. 2012;7:12244–53.

Winiarski J, Cie B, Kunicki P, Szczygie B. Applied Surface Science Corrosion of nanocrystalline nickel coatings electrodeposited from choline chloride : ethylene glycol deep eutectic solvent exposed in 0 . 05 M NaCl solution. Appl Surf Sci J. 2019;470(November 2018):331–9.

Chaoqun L, Xinhai L, Zhixing W, Huajun G. Mechanism of Nanocrystalline Nickel Electrodeposition from Novel Citrate Bath. Rare Met Mater Eng. 2015;44(7):1561–7.

Park K, Ahn S, Kwon H. Effects of solution temperature on the kinetic nature of passive film on Ni. Electrochim Acta. 2011;56(3):1662–9.

Nasirpouri F, Sanaeian MR, Samardak AS, Sukovatitsina E V., Ognev A V., Chebotkevich LA, et al. An investigation on the effect of surface morphology and crystalline texture on corrosion behavior, structural and magnetic properties of electrodeposited nanocrystalline nickel films. Appl Surf Sci. 2014;292:795–805.

Zamanzad-Ghavidel MR, Raeissi K, Saatchi A. The effect of surface morphology on pitting corrosion resistance of Ni nanocrystalline coatings. Mater Lett. 2009;63(21):1807–9.

Belhamel K, Kheraz H, Ludwig R, Nguen TKD, Allsop N, AL-Juaid SS. Electrodeposition and morphology analysis of nickel nanoparticles from sulphate bath. e-Journal Surf Sci Nanotechnol. 2010;8(May):227–32.

Wasekar NP, Haridoss P, Seshadri SK, Sundararajan G. Influence of mode of electrodeposition, current density and saccharin on the microstructure and hardness of electrodeposited nanocrystalline nickel coatings. Surf Coatings Technol. 2016;291:130–40.

Rashidi AM. A Galvanostatic Modeling for Preparation of Electrodeposited Nanocrystalline Coatings by Control of Current Density. J Mater Sci Technol. 2012;28(12):1071–6.

Liu M, Liu H, Wang D, Liu B, Shi Y, Li F, et al. Effect of nanodiamond concentration and the current density of the electrolyte on the texture and mechanical properties of Ni/Nanodiamond composite coatings produced by electrodeposition. Materials (Basel). 2019;12(7).

Seo MH, Kim DJ, Kim JS. The effects of pH and temperature on Ni-Fe-P alloy electrodeposition from a sulfamate bath and the material properties of the deposits. Thin Solid Films. 2005;489(1-2):122–9.

Zhu YL, Katayama Y, Miura T. Effects of coumarin and saccharin on electrodeposition of Ni from a hydrophobic ionic liquid. Electrochim Acta. 2014;123:303–8.

Zhu YL, Katayama Y, Miura T. Effects of acetone and thiourea on electrodeposition of Ni from a hydrophobic ionic liquid. Electrochim Acta. 2012;85:622–7.

Zaki Ahmad. • ISBN: 0750659246 • Pub. Date: September 2006 • Publisher: Elsevier Science & Technology Books. 2006.

Aydin G, Yazici A. Effect of quenching and tempering temperature on corrosion behavior of boron steels in 3.5 wt.% NaCl solution. Int J Electrochem Sci. 2019;14(3):2126–35.

Kang W, Gao Z, Liu Y, Wang L. Effect of flow rate on corrosion behavior and hydrogen evolution potential of X65 steel in 3.5% NaCl solution. Int J Electrochem Sci. 2019;14(3):2216–23.

Tang J, Hu Y, Wang H, Zhu Y, Wang Y, Nie Z, et al. Complicated synergistic effects between three corrosion inhibitors for Q235 steel in a CO 2 -saturated 3.5 wt% NaCl solution. Int J Electrochem Sci. 2019;14(3):2246–64.

Fattah-alhosseini A, Naseri M, Gashti SO, Vafaeian S, Keshavarz MK. Effect of anodic potential on the electrochemical response of passive layers formed on the surface of coarse- and fine-grained pure nickel in borate buffer solutions. Corros Sci. 2018;131(November 2017):81–93.

Gu C, Lian J, He J, Jiang Z, Jiang Q. High corrosion-resistance nanocrystalline Ni coating on AZ91D magnesium alloy. Surf Coatings Technol. 2006;200(18-19):5413–8.

Gu CD, You YH, Yu YL, Qu SX, Tu JP. Microstructure, nanoindentation, and electrochemical properties of the nanocrystalline nickel film electrodeposited from choline chloride-ethylene glycol. Surf Coatings Technol. 2011;205(21-22):4928–33.

Trompette JL, Massot L, Vergnes H. Influence of the oxyanion nature of the electrolyte on the corrosion/passivation behaviour of nickel. Corros Sci. 2013;74:187–93.

Iida M, Ohtsuka T. Ellipsometry of passive oxide films on nickel in acidic sulfate solution. Corros Sci. 2007;49(3):1408–19.

Ni H, Li P, Wang Z, Zou Z, Zhao M, Wang L, et al. Fabrication and characterization of nanocrystalline nickel with a grain size gradient by direct current electrodeposition. Int J Electrochem Sci. 2019;14(9):8429–38.

Бܗ QINL, Jian-she L, Qing J. Effect of grain size on corrosion behavior of electrodeposited bulk nanocrystalline Ni. Trans Nonferrous Met Soc China. 2009;20(1):82–9.

Yang Z, Liu X, Tian Y. Fabrication of super-hydrophobic nickel film on copper substrate with improved corrosion inhibition by electrodeposition process. Colloids Surfaces A Physicochem Eng Asp. 2019;560(October 2018):205–12.

Jinlong L, Tongxiang L, Chen W. Effect of electrodeposition temperature on grain orientation and corrosion resistance of nanocrystalline pure nickel. J Solid State Chem. 2016;240:109–14.




DOI: http://dx.doi.org/10.36055/fwl.v2i1.7724

Refbacks

  • There are currently no refbacks.